Showing posts with label neutron. Show all posts
Showing posts with label neutron. Show all posts

Thursday, August 17, 2017

Neutron Activation of Manganese Using Am-241 and Beryllium



Neutron Activation of Manganese Using Am-241 and Beryllium 


Here's a quick little neutron oven I piled together.



Radioisotope AM-241 gives off alpha radiation.

Beryllium hit by alpha radiation gives off neutrons.

Neutrons hit Manganese which gets irradiated and changed--also giving off gamma radiation.

Gamma radiation serves as the indicator that activation has taken place.






Our victim: good of Manganese Dioxide. It's a black power. I put some in a zip lock baggie for the test. Underneath the bottle is some hdpe plastic. Not really needed, but it's important to note that some elements need slowed down thermal neutrons to be activated. Supposedly, Manganese can be irradiated by fast (unmoderated) neutrons--thus I don't really need the hdpe plastic to slow them down, but what the heck: I've got tons of moderators: hdpe, paraffin wax, wax with boron in it, etc.






Final cap containing additional AM-241.




Various Am-241 sources piled on top of a piece of beryllium. The beryllium came from a defunct x-ray machine.




Awesome old ionizing smoke detector. It has 80 micro curies of Am-241 in it, instead of less than 1 micro curie like modern smoke detectors.



The unused portions (for my work) of the smoke detector.





Here's the cap portion of the smoke detector. So many people overlook this part, there are two little rectangular foil ribbons on the inside that are also AM-241!






Here's the big-boy AM-241 source. Yes, there are three sources in many of these big old smoke detectors!




The radioactive part is under the little cap at the top of this photo.





See that screw in the center? That's the adjustment screw that you can use to adjust how much AM-241 is exposed from the third AM-241 source when the smoke detector is in use.



Pyr-A-Larm (Pyralarm) smoke detector. This one is an F 3/5A and was just loaded with Americium 241 radioistope sources. Three in all! This is the "before" photo before I started disassembly.

These are always on eBay for $120, but sometimes they pop up for much, much less. Just be patient.


From reading the works of Carl Willis I found that radioactive manganese has a half life of about 2.5 hours, so you should let it irradiate in the neutron fluence for double that.

I'm not sure my gamma probe will be able to detect this low amount of gamma, so I may have to let the sample sit for a half-life or two in my gamma spectrometer setup.


Results to follow later and will be posted here. Busy at work and I don't have time to babysit a 5 hour gamma spectrometer run :)

Update: here's a pic of my gamma spectrometer after only two minutes. Notice the huge peak at 823mev! Success!!




Tuesday, June 9, 2015

My Radioactive Dime





My Radioactive Dime






Alpha particle hits aluminum.

Aluminum releases neutrons.

Neutrons hit silver dime and turns it radioactive.

Silver dime releases gamma radiation.



Alpha particles turn Aluminum-27 to phosphorus-30 (*see footnote)

This is accompanied by awesomely unique neutron radiation. 

What's so great about neutrons? They can transmute elements by sticking to them and changing them, sometimes making them radioactive. Remember: alpha, beta, gamma and x-ray radiation stops when the source is taken away. Turn off an x-ray machine and it's safe to walk into the room. Turn off the microwave oven and you can stick your hand safely inside to get out your nice warm popcorn.

Neutrons are a tad different though: they can irradiate elements. Blast neutrons at silver and you get radioactive silver! Turn off the neutrons and the silver is still radioactive (for a couple minutes at least).


Neutrons turn Silver-107 to silver-108 with a half life of about 2.5 minutes.

Neutrons turn Silver-109 to silver-110 with a half life of about 25 seconds.

Each of these reactions is followed by a lovely blast of easily detectable gamma radiation.

All that sounds a little fancy, how hard was it to accomplish in real life? Well, it was very simple really:

I wrapped an old silver dime in foil and left it in an alpha particle bath for a few days. I then carefully slide it next to a Geiger Counter that was shielded with paraffin wax. The baseline only mildly rose from 10cpm (clicks per minute) to 20cpm...but it did rise!

After less than two minutes it settled down to 6cpm.

10cpm was the normal background radiation in the room.
20cpm was the gamma released by the irradiated silver.
6cpm was the background radiation being partially blocked by the (now) back to normal nonradioactive silver.

Removing the silver let the rate go back to 10cpm.

These readings are very low all around, but repeatable. Back when dimes were silver the American Museum of Atomic Energy had a coin irradiating machine: pop in your dime and it would be made radioactive (for a couple minutes). Neat! But by the time you let the museum your dime transmuted back to being a boring old coin...which is good because who wants radioactive coins in their pocket?

It wasn't as momentous as when I finally got my nuclear cloud chamber working, but I did feel a little like Dr. Frankenstein and I proved my source has alpha radiation by inference since my Geiger Counter can only detect beta, gamma and x-rays...not alpha or neutron radiation; but I know both were there because of the increased gamma radiation driving up the cpm count.

Why the choice of materials used? Neutron cross sections. This tells us how interactive am element may be with neutrons. The larger the cross section the more reactive it will be. Cross sections are measured in units called "barns" which are ten to the negative twenty-fourth power in square centimeters (very, very tiny).

There are fast neutrons that can be slowed down by big scatter cross sections, and there are slowed "thermal" neutrons which can actually interact with things (like my silver dime) of those things have a big absorption cross section.

Elements/isotopes with large scatter cross sections and low mass are great neutron moderators (slower downers).

Aluminum scatters at 1.5barns and Silver absorbs at 91barns.

It's all starting to make sense isn't it!

The insanely poisonous metal Beryllium that I'm waiting for the mailman to bring me scatters at 7.6barns but only absorbs at 0.007barns...and it's the fourth element in the periodic table, meaning it had a relatively low mass. All this makes beryllium a fantastic thing to shoot alpha particles at and have it blast neutrons out in exchange!

What else is the mailman bringing me? Paraffin wax laced with Boron. Boron scatters at a respectable 5.24barns, but it absorbs at 767barns!! That will slow down lots of neutrons down to the thermal range, meaning those neutrons can actually interact better with things (my dime for instance).


This is all much more fun than using a Geiger counter that can see alpha, or a neutron detector.

Inference and implication. Pasteur said that fortune favors the prepared mind. I'll be building a zinc sulfide spinthariscope that lights up when an alpha particle hits it.

You can also modify a cheap webcam to see similar sparks when the imaging chip gets slammed into by an alpha particle.

I once had an old wristwatch. I noticed that it didn't glow steadily in the dark but twinkled. The next morning I researched it and found that it was painted with radioactive radium!

Neutrons can be detected by tubes filled with helium, lithium, boron trifluoride or a couple other pricey gases. There are also bubble dosimeters that show bubbles in a test tube where neutrons (or cosmic rays) pass through it.

Photo magnifying tubes are like night vision versions of the webcam method. Plastic scintillators light up with hit by particles-much like the spinthariscope method.

It's more fun inferring from chain reactions just like the discoverers did: a weird result that could only be explained by a previously unknown particle.

That's what you get from homemade "junk" versus fancy store bought lab equipment.

The inferences of a prepared mind. The fortune which befalls it via convoluted paths chance, accident or routine, simple experiments yeilding unexpected results that are tested instead of ignored.

Prepare your mind and fortune may follow.

*A footnote on the initial alpha and aluminum foil interactions: when the alpha particle hits the aluminum it makes phosphorus-30 plus a neutron. The phosphorus-30 decays into the usually stable silicon-30 by emitting positrons, but the silicon in this instance decays by emitting gamma radiation. The positron will likely slam into an electron and give off more gamma radiation.



Below is some great information on some older NEUTRON DETECTORS (as opposed to Geiger Counters) which you may find used online. I snagged most of this info from a 1973 report to the US Atomic Energy Commission by Alex Lorenz. If you want to read the full report, it's available as a PDF online by searching "Review of Neutron Detection Methods and Instruments".

That document has more information on each device, including the method of detection (i.e. chemical composition of scintillator crystal, etc.). It' a great document to consult if you're like many people and find just a part/tube/probe of one of these devices and want to use it with a different base/amplifier/etc.

You'll want to pay attention as to whether your Neutron detector sees fast or slow neutrons--that makes a difference in whether or not you need to use paraffin or other moderators or actually have to remove those barriers and moderators from your experiment. You don't want to slow down your neutrons with paraffin if your device can only see the fast ones and vice versa.  


DEVICE                         RANGE                       VOLTAGE

Ludlum Fast neutrons 900v
(Model 42-2)
Eberline slow or fast neutrons 900-1200v
(Model SPA-2)
Ludlum  1/v for thermal neutrons 900v
(Model 42-1)
Kaman thermal & fast — 120v
(Model A-300) 0-14 MeV
Ludlum thermal - 12 MeV 900v
(Model 42-4)
IiUdium thermal & fast neutrons 900v
(Model 42-5)
LND thermal neutrons ?
(Series 900)
Ortec ? ?
(System 525)
Nuclear Instruments  Linear between ?
and Chemical Corp. 10^7 and 10^12 nv
(Model 3782)
Reuter Stokes Co 1 0^15  nv ?
Reuter Stokes Cd 5X 0 ^014 nv ?
Reuter Stokes Rh 10^15 nv ?
Reuter Stokes V 10^15 nv ?
Reuter Stokes 10^10  nv 1000-1400v
(RSN-337)  (thermal)
Ludlum thermal and fast 500-2400v
(Model 15) neutrons
Centronics <7.5x10^10 nv 1000v
(Type D.C. 12)
Reuter Stokes 3x10^4 to 2.5x10^5 800-900v
(RSN-17A/326/ (thermal)
330/251/327)
Reuter Stokes 10^4 to 10^11 800v
(RSN-229A) (thermal)
Reuter Stokes 10^4 to 10^11 800v
(HSN-234A-M1) (thermal)
Reuter Stokes 10^3 to 10^10
(RSN-15A/304/ (thermal) 100-1000v
325/332/306)
Reuter Stokes 10^3 to 10^10 200-800v
(RSN-314A) (thermal)
Reuter Stokes 10^8 to 10^14 20-150v
(RSN-186S-M2 (thermal)
and 316S-M5)
LND 3 decades
(Series 30771) 500v
LND 5 decades  200-800v
(Series 3077) Thermal (U235) 
or fast (U238)
(Series 3075) Thermal 200-500v
 (Series 3000, Thermal 50-500v
Series 3050)
Centronics 9x10^3 to 9x10^7 250-500v
(PFC 16A)
Texas Nuclear Thermal 800-1400v
(Series 9300
Texlium)
Eberline Dose response from 1600-2000v
(PNR-4 and thermal to 10 MeV
NRD-1)
Eberline 0.01-10^3 eV & 1300-1800v
(PNC-4)  0.2-18 MeV
Harshaw Thermal 1700-3400v
(Model series
B3, B6, B12, B14)
Reuter Stokes 10^-3 to 10^-5 2500-3500v
(RSN-7A/7S/44/ Thermal
177S-M7/320-M2/
108S-MG)
N. Wood Model G ? 1100-2300v
Centronics 3.3x10^3 to 6x10^6 900-1100v
(Series 5EB/6)
Texas Nuclear Series 9300 Texlium Thermal 800-1400v
LND
(Series 3000, Thermal 50-500v
3050)
Centronics PFC 16A 9x10^3 to 9x10^7 250-500v
Centronics PFC 16B 10^11 200-400v




Phew! That was a LOT of typing! Enjoy!




Name      What is it?                                                                           Distance traveled 
                                                                                                                    through open air
Alpha       Physical particle equaling a Helium nucleus                        2-3cm

Beta          Physical particle equaling an electron                                    2-3m

Gamma    Not radioactive decay, just energy burst                                500m
                   accompanying alpha or beta radiation.
                   The same as an x-ray, but arising from
                   different sources.

Neutron     Physical particle made up of 1 up quark and                   1000s of meters
                     2 down quarks.


Name   Symbol     Makeup                           Charge         Speed       Atomic Mass Units
Alpha     α             2 protons & 2 Neutrons       + +                Slow                               4

Beta        β               1 electron                                -              Fast or Slow                1/2000

Gamma  γ                Photons/                           Neutral        Speed of light                   0
                           electromagnetic waves

Neutron n           1 up & 2 down quarks         Neutral      2.2km/S-14,000km/S         1
                                                                                                 (~5% speed of light)

Notes: 

An AMU (Atomic Mass Unit) is equal to 1/12 the mass of a Carbon-12 atom. 

Slow Neutrons are called "Thermal" and fast ones are called "Fast" neutrons. 

An alpha particle is double positive "++". 

Gamma rays are produced by atomic nuclei and x-rays are created by accelerating electrons, but they are basically the same type of wave energy. 


Lead only approximately halves the gamma/x-ray amounts. A 1/2" of lead stops about half the waves trying to get through. When beta radiation hits lead sometimes a new type of radiation is created that is more dangerous! This is Bremsstrahlung radiation (braking/deceleration). Lead barely interacts with neutron radiation, water or hydrogen-containing compounds such as common paraffin wax are much better shielding material.